Articles | Volume 1, issue 2
https://doi.org/10.5194/mr-1-315-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/mr-1-315-2020
© Author(s) 2020. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Research article
| 
17 Dec 2020
Research article |
| 17 Dec 2020
| 17 Dec 2020
Hyperfine spectroscopy in a quantum-limited spectrometer
Sebastian Probst
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Gengli Zhang
Department of Physics and The Hong Kong Institute of Quantum Information Science and Technology, The Chinese University of Hong Kong, Shatin, New Territories, Hong Kong, China
Miloš Rančić
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Vishal Ranjan
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Marianne Le Dantec
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Zhonghan Zhang
Chimie ParisTech, PSL University, CNRS, Institut de Recherche de Chimie Paris, 75005 Paris, France
Bartolo Albanese
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Andrin Doll
Laboratory of nanomagnetism and oxides, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Ren Bao Liu
Department of Physics and The Hong Kong Institute of Quantum Information Science and Technology, The Chinese University of Hong Kong, Shatin, New Territories, Hong Kong, China
John Morton
London Centre for Nanotechnology, University College London, London WC1H 0AH, UK
Thierry Chanelière
Univ. Grenoble Alpes, CNRS, Grenoble INP, Institut Néel, 38000 Grenoble, France
Philippe Goldner
Chimie ParisTech, PSL University, CNRS, Institut de Recherche de Chimie Paris, 75005 Paris, France
Denis Vion
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Daniel Esteve
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
Patrice Bertet
CORRESPONDING AUTHOR
Quantronics group, SPEC, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-sur-Yvette CEDEX, France
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Cited
17 citations as recorded by crossref.
- Electron-spin spectral diffusion in an erbium doped crystal at millikelvin temperatures M. Rančić et al. https://doi.org/10.1103/PhysRevB.106.144412
- Impact of Zeeman and hyperfine interactions on the magnetic properties of paramagnetic metal ions: II. Super-hyperfine interactions with surrounding nuclei Y. Kandrashkin https://doi.org/10.1016/j.jmr.2024.107732
- Electron-nuclear decoupling at a spin clock transition K. Kundu et al. https://doi.org/10.1038/s42005-023-01152-w
- Microwave Fluorescence Detection of Spin Echoes E. Billaud et al. https://doi.org/10.1103/PhysRevLett.131.100804
- Near-SurfaceTe+125Spins with Millisecond Coherence Lifetime M. Šimėnas et al. https://doi.org/10.1103/PhysRevLett.129.117701
- Transition Metal Ion Ensembles in Crystals as Solid-State Coherent Spin-Photon Interfaces: The Case of Nickel in Magnesium Oxide E. Poem et al. https://doi.org/10.1103/PRXQuantum.4.030329
- Towards telecom-compatible quantum nodes using erbium-doped stoichiometric EuCl3 ⋅ 6H2O crystals M. Guo et al. https://doi.org/10.1038/s41534-026-01203-4
- Electron and nuclear magnetic properties near ZEFOZ region Y. Kandrashkin https://doi.org/10.1016/j.jmr.2023.107433
- Opto-RF transduction in Er3+:CaWO4 T. Chanelière et al. https://doi.org/10.1016/j.jlumin.2024.120647
- Twenty-three–millisecond electron spin coherence of erbium ions in a natural-abundance crystal M. Le Dantec et al. https://doi.org/10.1126/sciadv.abj9786
- Impact of Zeeman and hyperfine interactions on the magnetic properties of paramagnetic metal Ions: I. Local interactions of the electron spin Y. Kandrashkin https://doi.org/10.1016/j.jmr.2024.107728
- Precision multi-mode microwave spectroscopy of paramagnetic and rare-earth ion spin defects in single crystal calcium tungstate E. Hartman et al. https://doi.org/10.1063/5.0224102
- A new anticrossing region of monoisotopic impurity 53Cr ions in Y2SiO5 R. Zaripov et al. https://doi.org/10.1016/j.jmmm.2025.172956
- Quantum sensing of a coherent single spin excitation in a nuclear ensemble D. Jackson et al. https://doi.org/10.1038/s41567-020-01161-4
- Adiabatic Control of the Phase Memory Relaxation in the Anticrossing Region Y. Kandrashkin https://doi.org/10.1007/s00723-024-01714-3
- Spectroscopic investigations of Pr3+:CaWO4 at liquid-helium temperatures T. Yang et al. https://doi.org/10.1103/PhysRevA.107.022802
- Large Hyperfine Coupling Arising from Pseudo-2S Ground States in a Series of Lutetium(II) Metallocene Complexes D. Ngo et al. https://doi.org/10.1021/jacs.5c01947
17 citations as recorded by crossref.
- Electron-spin spectral diffusion in an erbium doped crystal at millikelvin temperatures M. Rančić et al. https://doi.org/10.1103/PhysRevB.106.144412
- Impact of Zeeman and hyperfine interactions on the magnetic properties of paramagnetic metal ions: II. Super-hyperfine interactions with surrounding nuclei Y. Kandrashkin https://doi.org/10.1016/j.jmr.2024.107732
- Electron-nuclear decoupling at a spin clock transition K. Kundu et al. https://doi.org/10.1038/s42005-023-01152-w
- Microwave Fluorescence Detection of Spin Echoes E. Billaud et al. https://doi.org/10.1103/PhysRevLett.131.100804
- Near-SurfaceTe+125Spins with Millisecond Coherence Lifetime M. Šimėnas et al. https://doi.org/10.1103/PhysRevLett.129.117701
- Transition Metal Ion Ensembles in Crystals as Solid-State Coherent Spin-Photon Interfaces: The Case of Nickel in Magnesium Oxide E. Poem et al. https://doi.org/10.1103/PRXQuantum.4.030329
- Towards telecom-compatible quantum nodes using erbium-doped stoichiometric EuCl3 ⋅ 6H2O crystals M. Guo et al. https://doi.org/10.1038/s41534-026-01203-4
- Electron and nuclear magnetic properties near ZEFOZ region Y. Kandrashkin https://doi.org/10.1016/j.jmr.2023.107433
- Opto-RF transduction in Er3+:CaWO4 T. Chanelière et al. https://doi.org/10.1016/j.jlumin.2024.120647
- Twenty-three–millisecond electron spin coherence of erbium ions in a natural-abundance crystal M. Le Dantec et al. https://doi.org/10.1126/sciadv.abj9786
- Impact of Zeeman and hyperfine interactions on the magnetic properties of paramagnetic metal Ions: I. Local interactions of the electron spin Y. Kandrashkin https://doi.org/10.1016/j.jmr.2024.107728
- Precision multi-mode microwave spectroscopy of paramagnetic and rare-earth ion spin defects in single crystal calcium tungstate E. Hartman et al. https://doi.org/10.1063/5.0224102
- A new anticrossing region of monoisotopic impurity 53Cr ions in Y2SiO5 R. Zaripov et al. https://doi.org/10.1016/j.jmmm.2025.172956
- Quantum sensing of a coherent single spin excitation in a nuclear ensemble D. Jackson et al. https://doi.org/10.1038/s41567-020-01161-4
- Adiabatic Control of the Phase Memory Relaxation in the Anticrossing Region Y. Kandrashkin https://doi.org/10.1007/s00723-024-01714-3
- Spectroscopic investigations of Pr3+:CaWO4 at liquid-helium temperatures T. Yang et al. https://doi.org/10.1103/PhysRevA.107.022802
- Large Hyperfine Coupling Arising from Pseudo-2S Ground States in a Series of Lutetium(II) Metallocene Complexes D. Ngo et al. https://doi.org/10.1021/jacs.5c01947
Saved (final revised paper)
Latest update: 04 Oct 2026
Short summary
Electron spin detection was recently demonstrated using superconducting circuits and amplifiers at millikelvin temperatures, reaching the quantum limit of sensitivity. We use such a setup to measure electron-spin-echo envelope modulation on a small number of electron spins, in two model systems: bismuth donors in silicon and erbium ions doped in CaWO4 (calcium tungstate). Our results are a proof of principle that hyperfine spectroscopy is feasible with these quantum-limited ESR spectrometers.
Electron spin detection was recently demonstrated using superconducting circuits and amplifiers...
