Magnetic Resonance
Magnetic Resonance
MR
Articles | Volume 4, issue 1
Articles | Volume 4, issue 1
https://doi.org/10.5194/mr-4-27-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/mr-4-27-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
Articles | Volume 4, issue 1
Research article
 | 
08 Feb 2023
Research article |  | 08 Feb 2023

The effect of the zero-field splitting in light-induced pulsed dipolar electron paramagnetic resonance (EPR) spectroscopy

Andreas Scherer, Berk Yildirim, and Malte Drescher

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Latest update: 16 Sep 2025
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Short summary
Light-induced pulsed dipolar EPR spectroscopy (PDS) is an emerging field that uses photoexcited triplet states to determine distance restraints in the nanometer range. To date, light-induced PDS data have been analyzed with methods developed for techniques that do not invoke light-induced triplets. Here, we provide a new theoretical description that takes the full nature of the triplet state into account and demonstrate that it leads to more accurate fits of experimental data.
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